Triple coincidence measurement of the correlated electron momenta for strong-field double ionization
Time:2014-01-21ClickTimes:
Completely understanding of the dynamics of three-body Coulomb system, i.e.,
non-sequential double ionization, is a challenging task and represents one of
incompletely solved problems of theoretical and experimental physics, holding a
variety of puzzles on both classical and quantum levels. It is of paradigmatic
importance since it reveals complicated and fundamental electron dynamics in
atomic and molecular physics. Especially, the liberation of two or more
electrons from an atom by strong laser fields is dominated by the electron
correlation. Extensive studies of atoms and molecules in strong infrared light
fields have revealed that electron correlation dominates the enhancement of
double ionization yields at moderate laser intensity. Much effort has been
concentrated on exploring physical mechanism of strong-field non-sequential
double ionization.
Recently, Prof. Yunquan Liu and Prof. Qihuang Gong experimentally
collaborated with Prof. Ullich at Max-Planck-Institute for Nuclear Physics, and
have performed a triple coincidence study on differential momentum distributions
of strong-field double ionization of Ar atoms in linearly polarized fields (795
nm, 45 fs, W/cm2). Using a three-dimensional two-electron atomic-ensemble
semiclassical model including the tunneling effect for both electrons, we
retrieve differential momentum distributions and achieve a good agreement with
the measurement. Ionization dynamics of the correlated electrons for the
side-by-side and back-to-back emission is analyzed separately. According to
semiclasscial model, we find that the doubly excited states are largely
populated after the laser-assisted recollision and large amounts of double
ionization dominantly takes place through sequential ionization of doubly
excited states at such low laser intensity. This work has provided the complete
characterization of strong-field double ionization and was published on Phys.
Rev. Lett. 112,013003(2014) (http://prl.aps.org/abstract/PRL/v112/i1/e013003).
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Fig. 1. (a) The momentum conservation spectrum measured by the triple
coincidence. The experimental longitudinal momentum distributions of the fast
electron and slow electron of the side-by-side emission for positive momenta (b)
and for negative momenta (c), and of the back-to-back emission (d).
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We acknowledge the supports from the National Program on Key Basic Research
Project. Yunquan acknowledges the support by the National Science Fund for
Distinguished Young Scholars in China.